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In a small bowl or measuring glass, combine the strained berry puree, 1/4 cup simple syrup, and water with half the lemon zest and 2 tablespoons lemon juice.
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In the pitcher of your blender (you could also use a mixer), combine the buttermilk, cream cheese, 5 tablespoons simple syrup, and the remaining lemon zest and juice.
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To make stripes, pour 1 - 2 tablespoons of the berry mixture into the bottom of each mold and freeze for an hour. Next, add a layer of the buttermilk mixture and freeze for another hour. Repeat, until you’ve used all of both. Add the popsicle sticks after the second layer has set up a bit. Keep the berry puree and buttermilk mixtures in the fridge while the layers cure. Once popsicle molds are full, freeze popsicles overnight for a solid cure. I also found that the popsicles got even colder when frozen outside of their molds. Finally, I froze my popsicles on a tilt to achieve diagonal stripes, so give that a try if you’d like.
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If stripes aren’t your thing, divide the berry mixture between the molds, freeze for 30 minutes, pour in the buttermilk mixture, add the sticks, and freeze overnight.